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MAY RESEARCH REPORT 1965 Coatings and Resins Group CONFIDENTIAL /) HD0<*3 6 17 TRADE SALES MISCELLANEOUS Subject: S( Nptre2d3CSi ?aDtAin26"5Pjreservative Study May, 1965 Contributors: P. Hawkins, L. Taylor Summary: To find effective, inexpensive, non-toxic preservatives for Spred Satin, several preservatives, at various levels of concentrat~ion, were substituted for Dowicide A and Metasol L in Y-34l8 Decorator White, Discussion: Stability and preservative effectiveness tests of the following are now in progress. Concentration figures are based on total paint and represent the sum of the pre servative placed in the grind and the amount contributed by the thickener preservative: Troysan 1*12, Troy Chemical Co... and Fungitrol 11, Nuodex Products Co. - 0.012J6, O.O6256, 0.09^*, 0.11256, 0.26256; Biocide 280, Drew Chemcial Co. - O.OO656, 0.019#> 0.05756*, 0.06556, O.IO6J6; Nalcon 240 and Nalcon 248, Nalco Chemical Co. - 0.005J6, 0.02556, 0.064J6*, 0.045*6, 0.06556. An asterisk (*) after a concentration figure indicates standard 197-T-27A thickener was used In the let-down of the sample. /" Subject: All samples appear normal at this time. j Exposure Test No. 131: Corrosion Resistant Primers for Trade Sales Exposed: Cleveland - 45 South - 6 months Subject: Results: At this time the best primers are Y-471 and Y-1851-K. Y-585 and Y-I85I-L are a trace poorer. Next comes Y-470, then a Dyphos PO primer, the Y-I851 containing P-7 Lead, and finally an ex perimental Rustmaster Consumer White Primer con taining P-7 Lead. All paints are rated good for corrosion resistance at the scribe with the exception of the experimental primer which is fair. Exposure continuing. Exposure Test No. 79? Polyurethane Florenamel Tinting Base Exposed: Cleveland - 45 South - 12 months C7L0006637 Results: Color and gloss retention of Y-880 with 8 oz. per gallon tints of blue and ferrite dramatone are acceptable to good. Exposure continuing. Subject: Exposure TeBt No. 13*1: Medium Chrome Yellows Exposed: Cleveland - 45 South - 6 months Results: Regal X-3218 is equal to standard YW-2 for color retention, tint retention, and gloss. The Regal X-2778 is equal for gloss but slightly poorer for color and tint retention. Exposure con tinuing. Subject: Exposure Test Mo. 146: Complaint Investigation - BL-74 Fading Exposed: Cleveland - 45 South - 5 months New Orleans - 45 South - 3 months Results: Complaint of 2 month color fade - loss of BL-74, was not substantiated by these exposures. Sub stantiated by these exposures. Subsequent information supplied cause of complaint - there fore exposure discontinued. Subject: TlOp TM2`5004lK154 j Contributors: 3. Southwick, J. Bednarik / Summary: British-Titanlum Pigments "Tloxide R-CR3" We have made an initial examination of Tioxide R-CR3 versus Zopaque R-88-S. Our testing was in Japalac Enamel - Tint ing White (Y-1218-A). Two lots of R-88-S, two lots of RCR3, and a single lot of DuPont R-900 were evaluated. The R-CR3's were examined at three levels: an equal replacement of the R-88-S, a 95% replacement, and a 90^ replacement. Exterior exposures at Cleveland and New Orleans have been initiated and Weatherometer exposure is starting on these paints and gray tints of these tinting whites. Initial examination shows the Tioxide R-CR3 to be equal to R-88-S for hiding and tint strength at a 90-92.5j6 replace ment level. At this level improved gloss, appearance, and a noticeably bluer-cleaner tint tone is also observed. The Tioxide R-CR3 seems to be equal to DuPont R-900 for hiding, tint strength and tint tone. g U>006638 113 v The spectrum of this sample is an exact match for the Bpectrum obtained on Dion-6325 Polyester (reported 2-17-65) * Includes Fumaric 6.) Japco-9660 Pipe Coating (Jamestown P.&V. Co.) -- Madison DRIES; Lead (small calcium content was found, also) SOLVENT: Mineral spirits, xylene, super V, M, & P, naphtha, methyl ethyl ketone. BINDER. An unmodified, P. E. - glycerine - soya - o-phthalic alkyd. SOLVENTS BINDER CONSTANTS s-43 S-23 S-342 S-120 6956 856 21.5$ 1.556 P.A. 23.456 Soya F.A. 64.4# NV Acid No. 4o.4# 4.9# 7) 118-605 Light Chrome Yellow Amer-Fllnt (Am. Lacquer Solvents))-- Elmwood SOLVENT; Xylene, toluene, isopropanol, cellosolve acetate, ethyl acetate PIGMENT; Light chrome yellow (lead chromate - lead sulfate), silicates, silica BINDER; Epoxidized soyabean oil and cellulose acetate butyrate TOTAL SAMPLE PIGMENT / ) SOLVENT Pigment Solvent Binder 35.0# 29.356 35.7# BINDER PbCrOh PbS04 Silicates Silica 76.1# 14.2# 3*956 ^v3# CONSTANTS S-23 S-6 S-88 S-50 S-2 36.056 13.0# 12.856 1.1# > -- epoxidized soya ^76# C . A .B. ~24# NV Veh. NV 70.7# .9# 8.) 118-610 Catalyst (Am, Lacquer Solvents) -- Elmwood SOLVENTS; Xylene, Cellosolve Acetate SOLIDS: This is the Pentaerythritol esters of "Het" and phthalic acids (acids In large excess) NV Acid No Cl 33.556 158 (on NV) 30.256 (of NV) # Het. anly. 63.256 P.A. 23 . 456 SOLVENTS S-23 64.456 S-50 35.656 1 GLD006639 9.) #392 Clear Topcoat (Grand Rapids Varnish - for Plastlwall) -- Nubian SOLVENT; Toluene, methyl lsobutyl ketone, ispropanol, ethyl acetate, naphtha BINDER: Nitrocellulose, rosin-maleic adduct ester (such as VM-441), and a non-drying alkyd (saturated F.A. -- glycerine-- ophthallc alkyd). Fatty acid distribution (see below) is a good match for Neo-Fat #18-57 (hydrogenated tallow). No haze was observed when the sample was cooled (overnight'Tn a freezer, at -9F. both as is, and diluted 1 to 1 with S-6/ S-lll.) SOLVENT S-6 S-lll S-88 S-2 Naphtha 66.136 16.4# 12.6J6 2.9# 2.0J6 BINDER N.C. P.A. F.A. VM-441 & Polyol 33# 6# 27# balance FATTY ACIDS Myristic Palmitic Stearic Oleic 5.6# 30.3# 56.9# 7.2# CONSTANTS NV 29.1# N2 4.0# (of NV) 10.) Duracron #300 Modified Acrylic En. (C.P.I.) -- Toronto SOLVENTS: Toluene, butanol, xylene, naphtha (comparable to S-106), , methyf ethyl Ketone. /BINDER: The resin system here is essentially identical to a sample called Duracron #2591 Finishing Varnish (P. P. G. -- for Federal Tin), analyzed in September of 1963 for Elmwood. It consists of Duracron 200*, together with a substantial amount of high N.W. polypropylene glycol (such as Dow's P-2000). TOTAL SAMPLE Pigment Solvent Binder 17.3# 48.6# 34.3# SOLVENT _ CONSTANTS S-6 S-l S-23 S-106 S-120 Unk: 33.1# 32.6# 8.5# 21,4# 2.6# 1.8# NV Veh. NV vlh. Acid No. h 2o 51.6# 39-4# 2.0# 5.7# (14.5 on NV) 0.5# * Terpolymer of styrene (most), small amount of ester (very probably ethyl acrylate), and acrylamide formaldehyde, blended with an "Epon" type epoxy resin (present in fair amount). 11.) Arco En, Reduced for Electrocoating (Arco - for Gibson Refrig erator Co.) -- Nubian- 1 " s~~ SOLVENT: Toluene, xylene, methyl ethyl ketone, butan GLD006640