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AR226-2531 TO: B. TOW PPD Partersbur;g. W TA2LE IX Comparison of Ca/GC and Wickbold Torch Analyses of Rac Blood Sainnlaa^ a) PEAL So. 80-67461 80-67462 80-67752 80-67756 80-67481 80-67460 80-674S4 Sacetfice-Tubs 1-6 1-7 2-18 3-1S &-16 1-2 Tesi blank 5C Analysis, [C? 3, ^gJ/8 Mood 7.7 13.1 11. A -5 1.3 " I -- Jk <0.007 (none detected above rsagen; background) Wtckbold Torch Analysis, Total rluoride, M& F/g blood UatorrecCad it l/0.83<b) 6.9 8.3 10.5 12.7 9.5 11.4 9-0 10.8 1.5 2.2 I ; 1.3 3.7& 0.92 (a) Analyses cr. aur-ll-ca'-e scr^o^;- >:. She lyo^'hi.lizfcc bl=c'i saaylefr. G: ar.sly3e3 as descri?^--- .u; Tasle ;^;, 1Z-"..'^-:-12 S. 8C. ~'i=icfc'.'l= T;r--.-. 3-.3:.y-^ '--:. E- K.3S& .'ac^scn I.ab, ;; - Jl/tfC-l-""'31, Notfebc>-U eiarbr<:- ;90;-13^. ('b) Secovry ^.: ^srilucrooc^ana-lc -ici.:' ia ='ie Sickto;^ 7;--: ^'r- ;rc.:&:'-r ;?. cucre'ntly '-83S, as dacars-ned IE racsat -ork by ?. 'Sissz.. fi.in ^SES 99 0 EID951116 I I I TABLE . f \ ConcgntratLion of Perfluotooctanoate in Rat Blood Samples, GC Ucternltiatl.om8 "' Sacrifice I. 0 Days 2, 14 I>ays 3. 28 Days 4, 42 Itays 5, 8'i Iluya <.!tou|> 1 (coocrol) Tulie S (CnL UK F/B I I G r o u p Tube ff (1 ni^/B-') (Cal. 4g F/g I 0.68 6 7.7 2 1.1 7 13. 3 21. 8 17. 4 3.3 9 20. !> 0.53 10 9.4 Avc, 5.3 13 1.4 cxc.i 3 3 4 5 . 0.30 0.43 0.12 &ve. 0.28 3 0,086 a 0.97 4 0.11 9 1-.5 5 ; 0.11 10 0.84 Ave.. 0.10 1.2 1 U.OIO I O.Q37 I 0.058 ^ 0.038 5 0.017 Ave. 0.032 J 0.029 2 <.007 (c) 3 0.021 < <.rio? <c) i\vc. 0.0] 5 I I I Group Tube 1 (B ng/if') (CftL Ug F/K 11 53 i2 28 13 37 14 61 15 57 47 Group IV Tabe 1 16 17 18 19 20 ' 18 19 20 ' , 13 4.2 18 14 4.6 19 15 2.6 20 3.8 16 17 18 19 11 i 14 15 r,8zsoo2i"a TABUS III (con't) (a) Procedure as described in che method "Oetaniitttation of rerfluorooetanoic Acid in Blood Cas, Chroaa to graphic Machod", 1/2/81, using Cha capillary coluiBn GC analysis and partluoro-n-octanoic Add as calibration standard. Lowa,r lisas for quantication 0.007 ppm f. Eatlaiacad uacaTKSlniSy ^LOZ relative staadard deviation ovsr aosc of che range, somewhat higher at se lowest conceaeracicns. "wt (b) ror shfc six blank" sanples llatfld as analyzed in Tablo I, [Csl <0.007 ??ia ? (aone detected above reagent backsroiiid). (SAI. N05. 80-60368-69, 80-60372-75) (e) Values of 0.005 (saaple 5-2) and 0.003 (gafflpla 3-4) were used tc calculate the average, buE ^uaacltation cannot really be doofe at these levels, and 1C is questionable vhether 3-4 coataiaed any Cg above background. 042 42 iSS&S 99 e0 EID951118 TABLE IV Percitn':_Straight:-Chain Perflworpoct.anoate in Rac Blood Sanplea'*7 Sacrifice 1. 0 Day 2. 14 Bays 3, 28 Days ^ 42 Oaya 5, 84 Bays Tuba f 1 2 3 4 5 Percent 85 84 96 91 86 Tube (f 6 7 8 9 10 Percent 82 80 85 88 81 Tube 6 11 12 13 14 15 3 93 , 4 92 ! 5 91 - - * - 1 3 not 8 4 cal- 9 5 culasttd(b) 10 : 93 13 91 . 14 97 15 ----,----------i----------------------. 1 not 2 3 cal 4 5 culated (b) , -r 1 aot. 2 ' el- .' 3 ciil<ctd(b) & Prenc 89 92 90 85 86 Tub? ft 16 17 18 19 20 { 1 18 -| 1920 ! 96 . 18 95 ; 19 96 : 20 ''. 16 17 . . 18 ! 19 ', 1 ; 13 ,1415 Parcent 88 88 87 84 86 93 92 91 . 94 92 " 93 94 96 95 94 ^97 94 93 (a) Calculated as described- in the method, for peak 93 in tha group of five Cg Isooer peaks seen la Figur 3b. The ssaa calculation for iptked blood standards (^1Q ppn F) gave average values os 7^ acraigtie-cfaain for rc-143, 94X for pttrfluoro-n-Octanoic acid- (b) A calculation of branchftd laoaer concentrations vasooc accaniptad for saarolea with (Cgl^O.l ppa, due to the amail gi2i'of the secondardy paaka and incarference froffl ch4 reagents. 043 43 S N c> o <ji to 00 ^0 EID951119 Figure 1 ~ Comparison of Cg/GC and Wi.ck.bold Torch Analysts of fiat Blood Samples Data from Table 11, using Torch valuaa corracced for 83% recovery of perfluArooctanoic acid Linear Least Squares ric; Torch - 0.90 ' 0.9f (.GC) : --,'... ,!-^- '- '- i, --.. :-!' . - - -|P^'':'':l " i*- ri J- ! i. ! t . 1 : ...... - ; - i.* : -V 1 ! !. ----I---- -1 : ."!'' i !: ::"! .; i - ---- ' i r i -- > 1 i- 1 I ! 1 ] , " . ' / / S / / : ; : 1: ! : ' : - '. / Q- | > > I I ' i y / L.- ' 1 , i-- r-^Q i | \ '"! 1 ; . : ; . -ih^---r//-ip'ir/- \. Tor&h, Ii0 ; ,:;. 1 : .'!'!- : "! > . r . i - ~ E ' : f i 1" -" i >i ' ! ! .- '/' t^- \ ppm " ! F ^ ;:. * : - / y: ..'J = : : r; :; Y-- i i t : --.,,...: , . -: ~. r" - 1 ! :- .;; .. f i '' y i T -! t y:y\ / . 1 ! V ' '' \ : i "I i 1 1 ': ' . ; : : " ; s '' --- : s . 1. - i ' ; - ii ; /' .^ i-r :.l \ ..;.. -- - - r.r -.- i.- ^r \ \ ^ .1 : r ; ' : "; : ! ; ;: \ ' '' . :: 1 j"" .-- ! """ i ; --^ ^ i : - K-^-'-^-^-i- : [7-0-i~ j?j---- ---4- -J....-;.-.!'' a >< ! : </ ;< i>> ". ii ; t i J GC, ppa Cg as F N 0 0 044 - Ul 44 EID951120 ritur 2 - ConcM-tracton of Cg tn Itt Blood SaioplM v. Baccfry Tiaa Dat* (roa TabU Group IV & - Group III 0 - Croup II X - Gcovp I III, Avrg Vlw by flC . . lo C - I.? - 0.039 t (to 42 dty on-L?) lo( C - 1.7 - 0.039 t Xo C * 1.1 - 0.038 S '- log C ' D.0?8 - 0.0.33 6 <to A3 (biy only, ispl . 3-2,0 - Axc, lu.dti^l/ 45 EID951121