Document RVk9rrDGBMBokZKxvX549Z17

CAL B .U L l E T I N . ''p * * | % > T !> 9 . r> y; i i Hdi-iuii&o * ' : A series of inert, chomically-resistant, fire-retarding ' ; plasticizers compatible with wide variety of resins. li r j . TECHNICAL BULLETIN O/PL-308A *. ' i { v' w. *'>*. ' 'W*,. .v4--.tr.*t. At.**,*?V `'-> ' * ' V 0520J76 TOWOLDM6N0035994 AROCIOR PLASTICIZERS A series of inert, chemically-resistant, fire-retarding plasticizers compatible with wide variety of resins. TECHNICAL BULLETIN O/PL-306A . CAUTION: a*;. auction.; eritnlvQ Tojclci`y and Safa HaftdlinQ.and Environmental Haxxards, on paga \Z. 'r- .k< .*< i`tiMi'1 r 4uw( :* j (*: tti.vir.Mjfc's.Mi lumttvt *>taa*ut rr or A*Y MQC-UCn ..tfmiO 1l> <- z.*n ... .! >M<t;c(.rf ffwiti X- - xliMi k> cw UUeAMh-iMtmo<<*c*mrTLtMi(Mrf> am <.<*)>)?** *!.'* Organic Chemical* Dhfl*ioo/0Q N. ItAdbtrgfc fclvd./St. U!o, Mituun 6316ft 0530577 TOWOLDMON0035995 Introduction . '' . Solubility The unique Aroclor*1 plasticizers are among the most versatile chemi cally produced materials available. One outstanding characteristic -- . inertness -- makes Aroclor useful in malty was* tor many different applications. The major benefits offered by Aroc >r include: ' Chemical Resistance - Fire Retardance . Compatibility v. illt most resins Nonaxidation Adhesivity . Low Cost Monsanto's Aroclor plasticizers comprise a ser-s of chlorinated bi phenyls and chlorinated polyphenyls. They v;.-y from mobile, oily liquids to white crystals and hard, transparent rosins. Twelve of the Aroclor plasticizers, each of which represents a series, are discussed in this bulletin. An understanding of the system for designation of each Aroclor should prove useful m the evaluation of the property gradations among them. The last two digits indicate the approximate weight frcrcentage of chlorine in the product, and the first two digits indicate the type of material, as follows: . 12 -- chlorinated biphenyls ' 25 -- blend of cn'orinated biphenyls and . hlorinated triphcnyls (75:25) 44 -- blend of chlorinated biphenyls and ' hlorinated triphenyls ' (60:40) 54 -- chlorinated triphenyis For nearly every Aroclor nv-ui ioned. a darker, icss-pure grade exists,' with about"the su.,".r j,h.% steal ..r.d cl.envcai cha, acteristias, but lower in ppce. . The Aroclor liquids and resins are readily soli hie in most common organic solvents and drying oils. Although all A"ocior plasticizers are - insoluble in water, ibara. Tystaiiine muter is are generally less soluble than the liquids and softer resins. Solub; ities of some Aroclor plasticizers arc shown in Table 1. TOWLDMON0035996 TABLE 1 SOLUBILITIES OF AROCLOR PLASTICIZERS IN VARIOUS SOLVENTS Solvent At?Av 1242 2VC. Hat A>'io Acetic Acid sS Oleic Acid ' s g A till " Aio. Vi!;' 4C/' rof'aaJdehyt/e flJ.ifj' 11 VS VS Ann,5 Ani-'fis Fr^-jnc S 137V" s 44f|5?*c C^ic^jcn/atives Amy c^endes - mixed CaiVn latrcchtoide Ch! .wAum * : iiirhhiic'e M .* I.' fu!iCii?pe Or!; i j:.chWnfov:v;ene Tfcwv.li'jictimuc Trichlorethane Trichlo.cthytcne Cry^riA Oil Tun: 0:! Ur. - J Oil S s s -- i. i. -.s s s s s s s S -- s s -- .S s s S s ter Am>l Acetate Butyl Acetate "CeJfosolvc"* Acetate Cottonseed Oii Oibuiy! Piitiiotate s s s s s s s s s s Afjcior 1248 2S'C Hot _ -- 10.0"" -- -- Arocbr 1254 zrc not ss ss --- 1111 vs vs vs vs . s .s -- -- 114'c 425t ssss ssss ssss -------- ssss ssss -------- ssss ssss s s. s s ssss ssss ssss ssss ssss ssss ssss Atoctcr 1265 Cold Hot __ ---- ---- i1 S3 ss ' ---- ---- Ss ---- Ss -- --1 ------ ---- ---- _ 1s Ss ss ---- ---- ss Arochr 4485 Cold Hot Aroebr $460 :rc ss s s vs ---- 1 11 V? vs -- -- -- vs vs vs vs -- vs vs vs vs vs vs vs vs vs vs vs vs vs vs vs vs vs vs vs vs vs vs vs vs H6 -- ~ -- - -- --. _ -- vs vs vs vs -- vs vs -- s VS ' -- s vs -- Diethyl FlithaUte s S s s s s --- Et:y* Acetate s s s s s s SS SS Ethyl Urtotc ssGsss 1 s ttiy!enc Glycol Diacetatfl s s s s s s -- _ Methyl Acetate s s s s s s SS SS I'liOiphate s s s s s s ---- Ether: Ftbyl Ether s s s s s s S. 2 s the A'c!a> Cartifc!' 224*' Celhsohs s Qrtiiplc j: Glycol - p.v'-Uili&'Ui Ethyl Ether 16.9n*c 30?t s - jr-33't vs s -- SS vs l?3t 25S2**' sss 1 1 --~--- SS B-'OT to*9*1 -- s s --. -- Hyd.'ota'Susi 6rizc:tc Gswhir*. Kerosene M`iii-rr.! Spirits Par,>!Im Pme f;:i Tulu-:nr lurp':nt:r5 Xyk-.ie vs vs vs vs 2.0!,*'c s vs vs vs vs vs , vs vs vs vs vs vs s 2.{1> s vs vs , vs vs vs vs vs vs vs vs vs S p' VS ; vs' vs vs vs vs vs vs -- s vs vs vs vs vs vs vs s s vs vs . vs ss ---- SS s ss ---- ss ss s .s ss Hi't'roxy inivatives A y* fv: 'hu Ethyl .V;cho: (3-AJ Gtyccrjne Methyl Alcohol Phenol -- 305a Kew.te. Avetonc Miscellaneous Cerlor OisoUirfe Nfticlinzenc Wafer s s 23.3' 1 J3-30-C $ s s S1.9re I 8S.5E="= S & SS Ss |I ---- -- -- --- 11 ---- ---- ---- ---- -II s s 1D2,>C i 15", SS s s s 28s*' 22.265DC s $ SS 1 1 1 -- SS 1 s SS 1' 1 -- s 1 ssss s s -- IIII1I I -- Insoluble SS -- SliQhtty SoIubl S-Soluble VS - Very Soluble. Fiourcs show srams ol Aiotlot per 100 milliliters of solvent at 25'C unless otherwise indicated. s vs s vs vs vs vs vs s. s SS s s- SS -- s-- s-- SS -- vs vs vs vs vs vs vs vs 0.0 s ss vs VS vs vs vs vs ss SS s SS -- 11 SS . -- ss ss vs vs vs " -- -- -- -- -- -- -- ~ -- -- 143 -- -- -- -- -- 142 -- 123 -- -- -- -- - -- 260 .-- - - 08SO2SO I ' . .. TABU 2 CHEMICAL AND PHYSICAL PROPERTIES OF REPRESENTATIVE AROCLGR PLASTICIZERS AND RESINS Piopiltf Appeetence Anoint mi Clear, mobile oil Arochr mt Clear, mobile oil Anclor mi Clear. mobile oil Arodor mi Clear, mobile oil Arochr nm light-yellow viscous liquid Color, maximum *100 APHA *100 APHA 100 APHA *100 APHA 100 APHA Ckhrim. percent . 20.5-21.5 31.5-32.5 42 - 48 54 Aridity, mg nCH/g, maximum 0.0H `0.014 0.015 0.010 *0.010 Moisture, ppm, maximum - An. Coefficient ot Expansion, cc/cc/'C 0.0C071 (15`-40'C) - 0.00073 (2S'-100*C) *50 0.00068 (25'-65,C) *50 0.00070 (25*-65'C) 50 0.00056 (25--65'C) Specific Crerfty *1.182-1.152 (25715.5'C) 1.270-1.280 (25715.5'C) '1.381-1.392 (25715.5'C) 1.405-1.415 (65715.5'C) 1.495-1.505 (65715.5*0) Density, pounds per gallon, 25'C 9.85 10.55 11.50 ' 12.04 12.82 Distilhiion Rungs, *C. corrected {ASTM 0 20. modified) 275-320 . 200-325 *' 325-366 340-375 365-390 Irspntethn loss. %. 100*C. 8 hours (ASTin D-6, mod.) I63`C, 5 noun 10-1.5 l.fl-1.5 0-0.4 3.0-3.6 0-0.3' 3.0-4.0 0-0.2 1.1-1.3 flash Point (Cleveland Open Cup), 'C 141-1S0 F 286-302 152-154 305-310 176-160 348-356 153.195 373-384 Nona to boiling point file Point (Cleveland Open Cup), "C 176 *F WO _ 238 160 None to point Nona to baiting point None to boiling point Pitt: Point (AST.M i 57), *C 1 (crystals) --33.$ --19 -7 10 *P 34 (crystals) -32 2 19.4 50 Softening Point (ASTM -23). 'C - - - - - ' 'f Refractive index, it 0-20 20*C 1.817-1.618 1.620-1.022 1.627-1.629 1.630-1.631 1.639-1.841 Viy.. wt*. Seconds SayjoJt Univ'rsoJ j (ASiM D-38) tdb . 33-41 ni: f 1 35-17 210-F (98.9'C)1 5o-3i ___________________________________ L - 44-51 1 52-92 30-41 | 42-50 j ________ [ 34-35 185-240 '73-30 36-37 1660-2500 260-340 44-48 TOWLDMON0035999 Arodor USD Jght-ytllsw. oft. ctictcy rttin 150 APHA 60 `0.614 '50 O.CDOS7 (20`-100`C) .'1.555-1.555 (30715.5`C) 13.50 385-420 0 0.1 0.5-0.8 tion to boiling point None to toilir.) point 31 88 1.847-1.649 Atodot tin Atodot 1441 Atodar 44SS Atodot ISS5 Atodot im Atodor no light-yellow sticky, viscous min CJoar yjilow sticky rosin *150 APHA 61.5-62.5 *2 NPA (molten) 42 Clear. light-yellow. resin *2 NPA (molten) 35 Slack, opaque, brittle reain _. Cleer. yellowtO'3mber, brittle resin or Hokes *2 NPA (molten) 65 ' 53.6-60.8 White to off-white powder `1.5 NPA (molten) 68 0.014 - O.G0054 (25'-65`C) 8.05 - 0.00123 (25`-S3*C) 0.05 - ' 0.00061 <25`-S5*C) 1.4 0X0065 (25*-$5*C) 0.05 - 0.00179 (2S*-124'C) 0.06 - 0.00067 (20M00*C) *1.572-1.583 (90715.5'C) 1.470 (25725'C) 1.670 (25725`C) 1.704 (25725`C) 1.670 (25725`C) 1.804-7.611 (25725`C) 13.72 ' 12.24 13.91 14.44 13.91 15.09 390-425 215-300 (4 mm. Hg) 230-32tr (4 mm. Hg) 280-335 (5 mm. Kg) 435-450 0-0.1 0.5-0.8 0.01 0.2 0-0.02 0.2-0.3 0.2 -0.3 0.03 0-0.06 0.1-0.2 Nona to boiling point 247 477 Nona lo boiling point Nona to boiling point >350 > 602 - Nonelo boiling acint 38-38 69 _ - 1.6501 1.6517 48 110 *46-52 115-126 r- *60-68 140-151 1.664-1.667 __ . .. *6-72 149-162 - None to boiling point None to boiling point None to boiling point None to boiling point `38-105 208-222 1.660-1.635 tcO-170 (hold 3Q2433 point) - 3200-4500 *72-73 609-850 iuc-T. trc) 36-100 SCO-403 60150 -- (200V; 130`C) --' -- 0*>20*z ^ TOWo`-Dm6Noo36o00 Density All the Aroeior plasticizers are heavier than water, a valuable property for many applications. Densities are shown in Figure 1. Specific Volume The specific volume of Aroeior 1248 at different temperatures is as follows: Tmfertlan m 0 100 200 300 400 soa 600 ' Aiochr 1248 Specific Volume tmllp) 0.674 0.699 0.726 0.755 0.730 0.823 0.870 0*20*83 TOWOLDMON0036001 Volatility The low vaporization loss of Aroclor plasticizers is ind icated in Table 3. TABIE 3 VAPORIZATION RATES OF AROCLOR PLASTICIZERS Rlasticiter (Surface area: 12JS sq. cm.) Aroclor 1ZZ1 Aroclor 1232 Wt. loss (l) .0.5125 0.2572 ' Exposure at 1QTC (hr.) 24 24 l/aporiial/oa Rata (qlsq. cm.lht.) 0.00174 0.000874 Aroclor 1242 ' 0.0S95 24 0.000338 . Aroclor 1243 . 0.0443 24 0.000152 (lorafiu'-il-S 0.0745 43 . 0.000128 Oioctyl phtholate . 0.0683 48 0.000117 Dalrex" 25 0.0266 24 0.000087 Aroclor 1254 0.0168 24 0.000053 Shall Buttex 20 . 0.0047 24 0.000018 Aroclor J2S2 0.0039 M. 0.000013 Aroclor 1230 0.0026 24 0.000008 Aroclor 4465 . 0.0064 72 0.000007 Aroclor 6442 0.0033 72 0.000004 Aroclor 5460 0.0032 72 0.000004 Trictetyl phosphate 0.0010 24 0.000003 It is concluded that the vaporization rates of Aroclor plasticizers -- especially the most widely used 1254 and 1260 -- compare most favorably with the similar constants of other plasticizers selected specifically for these tests because of their low vaporization rates. IMWmM MWtoM.'K, 052058* TO'/'/OLDMON0036002 Vapor Pressure The vapor pressures of several Aroclor plasticizers are indicated in. Figure 2 over the temperature range 150 to 300C. , ' e . -|x 10>T.*K fi|). 2 -- Vapor Pressures of Aroclor Plasticizers The estimated vapor p>assures of several Aroclor plasticizers at 100F nho'.vn in the following table were determined by extrapolation from the values shown in Figure 2. ApptoximtU Vepor Pressure olAiocfot Flattieaert . . Cstmile<l et JOT F (37.S' CJ Aroclor 1232 -0.0Q5 mm. Kg A:o:!o' 1242 D.001 mm. Hg Arcelor 1248 0.00037 mm. Hg Aroclor 1254 0.00006 mm. Hg 0520585 TOWLDMON0036003 The viscosities of the Aroclor plasticizers vary according to whether the bo.se materia! is a biphenyl or a polyphenyl and on the degree of chlorination. In general the low-chlorinated biphenyls have the lowest viscosities (Figure 3). Ob205B6 TOWOLDMON0036004 forfeit/ Ar.j Safe Handling hhththn At ordinary temperatures the Aroclor chlorinated polyphenyls have not presented industrial toxicological problems. The hazard of potential toxic exposure varies with their volatility: the lower-chlorinated, more.volatile ones present more of a potential problem from the standpoint of both inhalation and skin contact. When Aroclor plasticizers are used at elevated temperatures, engineering controls must be applied, either by the use of closed systems or by affective local-exhaust ventilation together with general workroom exhaust. Vapor of the liquid Aroclor plasticizers at room temperature should not bo breathed in a confined space, and no vapor of any Aroclor evolved at elevated temperatures should be allowed to be dispersed into the general workroom. Inhalation teats on animals indicate that the maximum safe concen tration of vapor is in the range of from 0.5 to 1.0 milligram of the lower-chlorinated Aroclor piaaticizers per cubic meter of air. The threshold limit values (maximum allowable concentration for an 8hour working day) set by the American Conference of Government Hygienists are 1.0 milligram of the lower-chlorinated Aroclor com pounds per cubic meter of air and 0.5 milligram of the more-highlychlorinatcd compounds, such as Aroclor 1254, per cubic meter of air. Skin Confect '' Schwartz patch tests on 200 volunteers showed that Aroclor 1254 was neither a primary skin irritant or a sensitizer. Prolonged or repeated skin contact with the Aroclor plasticizers must be avoided by the use of gloves and protective garments, because of the possible occurrence of a condition called chioracne. Although re ports of this condition caused by Aroclor are rare, it can be produced by excessive skin contact. If any Aroclor is spilled on the 3kin the skin should be-washed in the usual manner with a soap solution. A burn caused by contact with a hot Aroclor should be treated like any ordinary burr. Aroclor plasticizer achering to the burned area need not be removed immediately, unless treatment of the bum demands it, in which case either soap and water or repeated washings with a vegetable oil are recommended. 05*0587 TowldmoNoo36005 [nvimmntal Hands Aroclor 1232, Aroclor 1242, Aroclor 1248, Aroclor 1254, Aroclor 1260, Aroclor 1262, Arodor 1268, Arodor 4465, and Montar 1 all contain polychlorinated biphenyls (PCB) of various types and in varying amounts. PCB residues in small amounts have been found in the environment and some studies have indicated that they may be harmful to certain forms of animal life. Extreme care should therefore be taken by all users of PCB-containing products to prevent any entry into the environment through spills, leakage, use, disposal, vaporization or otherwise. Further,..the products in which PCB materials are used, or which are formulated using PCB materials as a component, should be given careful study to eliminate the possibility -that PCB might reach the environment as a result of use in a given application. Some specific applications where the use of PCB should definitely be avoided arc in paints and sealants for swimming pools, paints and waterproofing agents in siios and other buildings where food products for humans or animals are stored, and as a component of any container or wrapping used in the packaging of food products. 05Z05&8 TOWLDMON0036006 Shipping r Freight Classification Aroclor 1221, 1232,1242, Synthetic Resin, Liquid, NOIBN 1248, 1254, 1260, 1262 Rail Classification Aroclor 1268, 4465, ' 5442, 5460 Synthetic Resin, Other Than Liquid, NOIBN Truck Classification Aroclor 1268 Aroclor 4466, 5442, 6460 Synthetic Resin, Powder, NOI Synthetic Resin, Lumps or Solid Mass, NOI Shipping Regulations None Standard Containers Aroclor 1221' -- Aroclor 1232 Aroclor 1242, 1248,1254, 1260,1262 Aroclor 1268 Aroclor 4465 Aroclor 5442 Aroclor 6460 (flaked) Tank car, 520-lb. steel drum, 60-lb. can Tank car, 550-lb. steel drum, 50-lb. can Tank car, 600-lb. steel drum, 50-lb. can 200-lb. fiber drum, 25-lb. fiber drum 600-lb. steel drum, 50-lb. can 450-lb, steei drum, 50-lb. can 50-lb. bag 0520589 TOWC"-DMON0036007 DISTRICT SALES OFFICES ALL DIVISIONS Additional District Ollicei era maiataiaad by: Agricultural Division AKRON. 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MISSOURI 63J86 0520590 TOWOLDM